Tear metabolomics for the diagnosis of primary open-angle glaucoma


Por: M. BOTELLO-MARABOTTO, M. MARTINEZ-BISBAL, M. PIAZO-DURAN and R. MARTINEZ-MANEZ

Publicada: 1 jun 2024 Ahead of Print: 1 mar 2024
Resumen:
Primary Open-Angle Glaucoma (POAG) is the most prevalent glaucoma type, and the leading cause of irreversible visual impairment and blindness worldwide. Identification of early POAG biomarkers is of enormous value, as there is not an effective treatment for the glaucomatous optic nerve degeneration (OND). In this pilot study, a metabolomic analysis, by using proton (1H) nuclear magnetic resonance (NMR) spectroscopy was conducted in tears, in order to determine the changes of specific metabolites in the initial glaucoma eyes and to discover potential diagnostic biomarkers. A classification model, based on the metabolomic fingerprint in tears was generated as a non-invasive tool to support the preclinical and clinical POAG diagnosis. 1H NMR spectra were acquired from 30 tear samples corresponding to the POAG group (n = 11) and the control group (n = 19). Data were analysed by multivariate statistics (partial least squares-discriminant analysis: PLS-DA) to determine a model capable of differentiating between groups. The whole data set was split into calibration (65%)/validation (35%), to test the performance and the ability for glaucoma discrimination. The calculated PLS-DA model showed an area under the curve (AUC) of 1, as well as a sensitivity of 100% and a specificity of 83.3% to distinguish POAG group versus control group tear data. This model included 11 metabolites, potential biomarkers of the disease. When comparing the study groups, a decrease in the tear concentration of phenylalanine, phenylacetate, leucine, n-acetylated compounds, formic acid, and uridine, was found in the POAG group. Moreover, an increase in the tear concentration of taurine, glycine, urea, glucose, and unsaturated fatty acids was observed in the POAG group. These results highlight the potential of tear metabolomics by 1H NMR spectroscopy as a non-invasive approach to support early POAG diagnosis and in order to prevent visual loss.

Filiaciones:
M. BOTELLO-MARABOTTO:
 Univ Valencia, Univ Politecn Valencia, Inst Interuniv Invest Reconocimiento Mol & Desarro, Valencia, Spain

 Univ Politecn Valencia, Inst Invest Sanitaria La Fe IISLAFE, Unidad Mixta Invest Nanomed & Sensores, Valencia, Spain

 Inst Salud Carlos III, CIBER Bioingn Biomat & Nanomed, Madrid, Spain

:
 Univ Valencia, Univ Politecn Valencia, Inst Interuniv Invest Reconocimiento Mol & Desarro, Valencia, Spain

 Univ Politecn Valencia, Inst Invest Sanitaria La Fe IISLAFE, Unidad Mixta Invest Nanomed & Sensores, Valencia, Spain

 Inst Salud Carlos III, CIBER Bioingn Biomat & Nanomed, Madrid, Spain

 Univ Valencia, Dept Quim Fis, C Doctor Moliner 50, Valencia 46100, Spain

M. PIAZO-DURAN:
 Ophthalm Res Unit Santiago Grisolia FISABIO, Valencia, Spain

 Univ Valencia, Cellular & Mol Ophthalmobiol Res Grp, Valencia, Spain

 Inst Hlth Carlos III, Spanish Net Inflammatory Res REI RICORS RD21 0002, Madrid, Spain

R. MARTINEZ-MANEZ:
 Univ Valencia, Univ Politecn Valencia, Inst Interuniv Invest Reconocimiento Mol & Desarro, Valencia, Spain

 Univ Politecn Valencia, Inst Invest Sanitaria La Fe IISLAFE, Unidad Mixta Invest Nanomed & Sensores, Valencia, Spain

 Inst Salud Carlos III, CIBER Bioingn Biomat & Nanomed, Madrid, Spain

 Univ Politecn Valencia, Dept Quim, Valencia, Spain

 Univ Politecn Valencia, Ctr Invest Principe Felipe, Unidad Mixta UPV CIPF Invest Mecanismos Enfermedad, Valencia, Spain
ISSN: 00399140





TALANTA
Editorial
ELSEVIER, RADARWEG 29, 1043 NX AMSTERDAM, NETHERLANDS, Reino Unido
Tipo de documento: Article
Volumen: 273 Número:
Páginas: 125826-125826
WOS Id: 001207615200001
ID de PubMed: 38479028
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